Milliwatt-scale 3D thermoelectric generators via additive screen printing
Energy Environ. Sci., 2025, Advance Article
DOI: 10.1039/D5EE01151E, Paper Open Access   This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.Sairam Antharam, Muhammad Irfan Khan, Leonard Franke, Zirui Wang, Nan Luo, Jan Feßler, Wenjie Xie, Uli Lemmer, Md Mofasser Mallick
This study reports an additive screen-printing method for a high-performance fully printed planar 3D TEG, achieving a milliwatt-scale power output of 1.22 mW at ΔT of 43 K, underlining its potential for battery-free IoT applications.
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DOI: 10.1039/D5EE01151E, Paper Open Access   This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.Sairam Antharam, Muhammad Irfan Khan, Leonard Franke, Zirui Wang, Nan Luo, Jan Feßler, Wenjie Xie, Uli Lemmer, Md Mofasser Mallick
This study reports an additive screen-printing method for a high-performance fully printed planar 3D TEG, achieving a milliwatt-scale power output of 1.22 mW at ΔT of 43 K, underlining its potential for battery-free IoT applications.
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One ultrasonic measurement for non-invasive and whole-life-cycle thermal diagnosis of lithium-ion batteries
Energy Environ. Sci., 2025, Accepted Manuscript
DOI: 10.1039/D5EE01892G, PaperLingshi Zhang, Zhongbao Wei, Chunxia Liu, Hongwen He, Kailong Liu, Guangmin Zhou, Yunhui Huang, Zhichuan J. Xu
Thermal characterization and diagnosis are critical for the whole-life-cycle safety of lithium-ion batteries (LIBs). However, conventional techniques are time-delayed and discontinuous due to the sealed structure and intricate mechanisms of...
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DOI: 10.1039/D5EE01892G, PaperLingshi Zhang, Zhongbao Wei, Chunxia Liu, Hongwen He, Kailong Liu, Guangmin Zhou, Yunhui Huang, Zhichuan J. Xu
Thermal characterization and diagnosis are critical for the whole-life-cycle safety of lithium-ion batteries (LIBs). However, conventional techniques are time-delayed and discontinuous due to the sealed structure and intricate mechanisms of...
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All-day freshwater and power generation via integrated photothermal-enhanced thermoelectrics and evaporation cooling
Energy Environ. Sci., 2025, Accepted Manuscript
DOI: 10.1039/D5EE02663F, PaperWenhe Zhang, Chengbing Wang, Lu Wang, Fan Wang, Puxin Tan, Jinchi Ma, Jingjing Jin, Zhongrong Geng, Hongyao Xie, Li-Dong Zhao
Solar-powered simultaneous electricity and freshwater production is a promising solution to address energy and water shortages. However, current technologies are limited by their reliance on sunlight and have yet to...
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DOI: 10.1039/D5EE02663F, PaperWenhe Zhang, Chengbing Wang, Lu Wang, Fan Wang, Puxin Tan, Jinchi Ma, Jingjing Jin, Zhongrong Geng, Hongyao Xie, Li-Dong Zhao
Solar-powered simultaneous electricity and freshwater production is a promising solution to address energy and water shortages. However, current technologies are limited by their reliance on sunlight and have yet to...
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Crack pinning enables stable cycling of micro-sized silicon anodes for wide-temperature lithium-ion batteries
Energy Environ. Sci., 2025, Accepted Manuscript
DOI: 10.1039/D5EE02997J, PaperKangjia Hu, Jiahui Zhang, Xinrun Yu, Jin-Bao Wang, Xianluo Hu
Silicon anodes promise revolutionary lithium-ion battery energy density, yet commercial viability remains constrained by catastrophic volume expansion and interfacial degradation under demanding thermal conditions. Here, we demonstrate engineered crack pinning...
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DOI: 10.1039/D5EE02997J, PaperKangjia Hu, Jiahui Zhang, Xinrun Yu, Jin-Bao Wang, Xianluo Hu
Silicon anodes promise revolutionary lithium-ion battery energy density, yet commercial viability remains constrained by catastrophic volume expansion and interfacial degradation under demanding thermal conditions. Here, we demonstrate engineered crack pinning...
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Promoting Sulfur Redox Kinetics of Atomically Dispersed Fe-NC Electrocatalyst by Carbon Vacancy toward Robust Lithium-Sulfur Batteries
Energy Environ. Sci., 2025, Accepted Manuscript
DOI: 10.1039/D5EE00262A, PaperJie Zhang, Dawei Yang, Canhuang Li, Qianhong Gong, Wei Bi, WEIHONG LAI, Shengjun Li, Yaojie Lei, Guangmin Zhou, Andreu Cabot, Guoxiu Wang
Single-atom catalysts (SACs) have become the key to overcoming the inherent limitations of lithium-sulfur (Li-S) batteries for their exceptional catalytic activity, high selectivity, and strong affinity towards lithium polysulfides (LiPSs)....
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DOI: 10.1039/D5EE00262A, PaperJie Zhang, Dawei Yang, Canhuang Li, Qianhong Gong, Wei Bi, WEIHONG LAI, Shengjun Li, Yaojie Lei, Guangmin Zhou, Andreu Cabot, Guoxiu Wang
Single-atom catalysts (SACs) have become the key to overcoming the inherent limitations of lithium-sulfur (Li-S) batteries for their exceptional catalytic activity, high selectivity, and strong affinity towards lithium polysulfides (LiPSs)....
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Transition pathways to electrified chemical production within sector-coupled national energy systems
Energy Environ. Sci., 2025, Accepted Manuscript
DOI: 10.1039/D5EE01118C, Paper Open Access   This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.Patricia Mayer, Florian Joseph Baader, David Yang Shu, Ludger Leenders, Christian Zibunas, Stefano Moret, André Bardow
The chemical industry's transition to net-zero greenhouse gas (GHG) emissions is particularly challenging due to the carbon inherently contained in chemical products, eventually released to the environment. Fossil feedstock-based production...
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DOI: 10.1039/D5EE01118C, Paper Open Access   This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.Patricia Mayer, Florian Joseph Baader, David Yang Shu, Ludger Leenders, Christian Zibunas, Stefano Moret, André Bardow
The chemical industry's transition to net-zero greenhouse gas (GHG) emissions is particularly challenging due to the carbon inherently contained in chemical products, eventually released to the environment. Fossil feedstock-based production...
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Exposing binding-favourable facets of perovskites for tandem solar cells
Energy Environ. Sci., 2025, Accepted Manuscript
DOI: 10.1039/D5EE02462E, Paper Open Access   This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.Junke Wang, Shuaifeng Hu, Zehua Chen, Zhongcheng Yuan, Pei Zhao, Akash Dasgupta, Fengning Yang, Jin Yao, MInh Anh Truong, Gunnar Kusch, Esther Hung, Nick R. M. Schipper, Laura Bellini, Guus J. W. Aalbers, Zonghao Liu, Rachel Oliver, Atsushi Wakamiya, Rene A J Janssen, Henry Snaith
Improved understanding of heterojunction interfaces has enabled multijunction photovoltaic devices to achieve power conversion efficiencies that exceed the detailed-balance limit for single-junctions. For wide-bandgap perovskites, however, the pronounced energy loss...
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DOI: 10.1039/D5EE02462E, Paper Open Access   This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.Junke Wang, Shuaifeng Hu, Zehua Chen, Zhongcheng Yuan, Pei Zhao, Akash Dasgupta, Fengning Yang, Jin Yao, MInh Anh Truong, Gunnar Kusch, Esther Hung, Nick R. M. Schipper, Laura Bellini, Guus J. W. Aalbers, Zonghao Liu, Rachel Oliver, Atsushi Wakamiya, Rene A J Janssen, Henry Snaith
Improved understanding of heterojunction interfaces has enabled multijunction photovoltaic devices to achieve power conversion efficiencies that exceed the detailed-balance limit for single-junctions. For wide-bandgap perovskites, however, the pronounced energy loss...
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All-solid-state batteries stabilized with electro-mechano-mediated phosphorus anodes
Energy Environ. Sci., 2025, Advance Article
DOI: 10.1039/D4EE05704J, PaperKaier Shen, Xuhui Yao, Huimin Song, Weize Shi, Chenxi Zheng, Xufeng Hong, Yingjing Yan, Xu Liu, Lujun Zhu, Yun An, Tinglu Song, Muhammad Burhan Shafqat, Chenyan Ma, Lei Zheng, Peng Gao, Yakun Liu, Mohammadhosein Safari, Yunlong Zhao, Quanquan Pang
An electro-mechano-mediation strategy was developed to enhance charge transport kinetics and mitigate the chemo-mechanical degradation of P anodes, which enables stable cycling of high-areal-capacity, all-solid-state lithium batteries.
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DOI: 10.1039/D4EE05704J, PaperKaier Shen, Xuhui Yao, Huimin Song, Weize Shi, Chenxi Zheng, Xufeng Hong, Yingjing Yan, Xu Liu, Lujun Zhu, Yun An, Tinglu Song, Muhammad Burhan Shafqat, Chenyan Ma, Lei Zheng, Peng Gao, Yakun Liu, Mohammadhosein Safari, Yunlong Zhao, Quanquan Pang
An electro-mechano-mediation strategy was developed to enhance charge transport kinetics and mitigate the chemo-mechanical degradation of P anodes, which enables stable cycling of high-areal-capacity, all-solid-state lithium batteries.
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Molecular engineering of D-glucuronamide additive directs (100)-oriented Zn deposition for ultra-stable zinc-ion batteries
Energy Environ. Sci., 2025, Advance Article
DOI: 10.1039/D5EE02101D, PaperLe Zhang, Shuyu Bi, Xijun Liu, Qiangchao Sun, Tao Hu, Xionggang Lu, Hongwei Cheng
An electrolyte additive D-Glucuronamide (D-Glu) functionalized with hydroxyl, carbonyl, and amide groups and a 3D architecture is introduced to co-modulate the thermodynamics and kinetics of zinc plating/stripping synergistically.
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DOI: 10.1039/D5EE02101D, PaperLe Zhang, Shuyu Bi, Xijun Liu, Qiangchao Sun, Tao Hu, Xionggang Lu, Hongwei Cheng
An electrolyte additive D-Glucuronamide (D-Glu) functionalized with hydroxyl, carbonyl, and amide groups and a 3D architecture is introduced to co-modulate the thermodynamics and kinetics of zinc plating/stripping synergistically.
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All-organic siloxane strengthening polymer dielectric for high-temperature capacitive energy storage at harsh-environment electronics
Energy Environ. Sci., 2025, Accepted Manuscript
DOI: 10.1039/D5EE01964H, PaperXiang Li, Kun Fan, Jingyi He, Siyuan Sun, Yinan Chai, Zhi-Min Dang, Xiangyang Liu
Dielectric polymer films often suffer from poor energy-storage level in harsh-environment electronic devices, circuits and systems. In this work, a molecular engineering strategy is described to synergistically achieve high mechanical...
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DOI: 10.1039/D5EE01964H, PaperXiang Li, Kun Fan, Jingyi He, Siyuan Sun, Yinan Chai, Zhi-Min Dang, Xiangyang Liu
Dielectric polymer films often suffer from poor energy-storage level in harsh-environment electronic devices, circuits and systems. In this work, a molecular engineering strategy is described to synergistically achieve high mechanical...
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Non-noble metal–organic frameworks in electrocatalytic urea-assisted hydrogen production and energy-saving regeneration
Energy Environ. Sci., 2025, Accepted Manuscript
DOI: 10.1039/D5EE02029H, Review ArticleSoheila Sanati, Rajender S. Varma, Min Liu, Reza Abazari
One of the unique features of urea is its non-toxicity and high hydrogen content, which makes it a very good candidate for the generation of hydrogen as a fuel. The...
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DOI: 10.1039/D5EE02029H, Review ArticleSoheila Sanati, Rajender S. Varma, Min Liu, Reza Abazari
One of the unique features of urea is its non-toxicity and high hydrogen content, which makes it a very good candidate for the generation of hydrogen as a fuel. The...
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Future Environmental Impacts of Global Iron and Steel Production
Energy Environ. Sci., 2025, Accepted Manuscript
DOI: 10.1039/D5EE01356A, Paper Open Access   This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.Carina Harpprecht, Romain Sacchi, Tobias Naegler, Mariësse van Sluisveld, Vassilis Daioglou, Arnold Tukker, Bernhard R.P. Steubing
The iron and steel industry is not only responsible for up to 9% of global greenhouse (GHG) emissions, but also associated with other environmental impacts. Anticipated growth in steel demand...
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DOI: 10.1039/D5EE01356A, Paper Open Access   This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.Carina Harpprecht, Romain Sacchi, Tobias Naegler, Mariësse van Sluisveld, Vassilis Daioglou, Arnold Tukker, Bernhard R.P. Steubing
The iron and steel industry is not only responsible for up to 9% of global greenhouse (GHG) emissions, but also associated with other environmental impacts. Anticipated growth in steel demand...
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Regulating segmental dynamics for ion clusters in polymer binders to realize high-areal-capacity electrodes in lithium batteries
Energy Environ. Sci., 2025, Advance Article
DOI: 10.1039/D5EE01785H, Paper Open Access   This article is licensed under a Creative Commons Attribution-NonCommercial 3.0 Unported Licence.Dong-Yeob Han, Sungryong Kim, Yeongseok Kim, Haeryang Lim, Gyeong Rok Lee, Chi Keung Song, Woo-Jin Song, Hong Chul Moon, Soojin Park, Taiho Park
Ionic soft polymers regulate the segmental dynamics of the side chains, forming reversible ion clusters. The ion clusters enhance Li+ conduction and electrode durability, realizing an ultrathick cathode for high-energy-density energy storage.
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DOI: 10.1039/D5EE01785H, Paper Open Access   This article is licensed under a Creative Commons Attribution-NonCommercial 3.0 Unported Licence.Dong-Yeob Han, Sungryong Kim, Yeongseok Kim, Haeryang Lim, Gyeong Rok Lee, Chi Keung Song, Woo-Jin Song, Hong Chul Moon, Soojin Park, Taiho Park
Ionic soft polymers regulate the segmental dynamics of the side chains, forming reversible ion clusters. The ion clusters enhance Li+ conduction and electrode durability, realizing an ultrathick cathode for high-energy-density energy storage.
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Breaking the limits of Ruddlesden-Popper cathodes to achieve a game-changer for proton-conducting solid oxide fuel cells
Energy Environ. Sci., 2025, Accepted Manuscript
DOI: 10.1039/D5EE00993F, PaperYanru Yin, Hongfang Huang, Samir Boulfrad, Hailu Dai, Yueyuan Gu, Shoufu Yu, Lei Bi
Ruddlesden-Popper (R-P) structured oxides are promising cathode materials for proton-conducting solid oxide fuel cells (H-SOFCs) due to their excellent thermal compatibility and chemical stability. However, the performance of R-P cathodes...
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DOI: 10.1039/D5EE00993F, PaperYanru Yin, Hongfang Huang, Samir Boulfrad, Hailu Dai, Yueyuan Gu, Shoufu Yu, Lei Bi
Ruddlesden-Popper (R-P) structured oxides are promising cathode materials for proton-conducting solid oxide fuel cells (H-SOFCs) due to their excellent thermal compatibility and chemical stability. However, the performance of R-P cathodes...
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Manipulating anion solvation competitiveness via a multifunctional additive toward robust low-temperature sodium metal batteries
Energy Environ. Sci., 2025, Accepted Manuscript
DOI: 10.1039/D5EE01919B, PaperTonghui Zhang, Ying Xiao, Shunshun Zhao, Yu Han, Gang He, Shimou Chen
The kinetic conflict between accelerated Na⁺ desolvation and durable interphase construction remains a bottleneck for sodium metal batteries (SMBs) operating at low temperatures. Herein, we propose an electrolyte engineering strategy...
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DOI: 10.1039/D5EE01919B, PaperTonghui Zhang, Ying Xiao, Shunshun Zhao, Yu Han, Gang He, Shimou Chen
The kinetic conflict between accelerated Na⁺ desolvation and durable interphase construction remains a bottleneck for sodium metal batteries (SMBs) operating at low temperatures. Herein, we propose an electrolyte engineering strategy...
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Three-Dimensional Bowl-Shaped Solid Additive Achieves 20.52% Efficiency Organic Solar Cells with Enhanced Thermal Stability via Curvature-Mediated Morphology Regulation
Energy Environ. Sci., 2025, Accepted Manuscript
DOI: 10.1039/D5EE01977J, PaperZhicheng Zhong, Sergio Gámez-Valenzuela, Jin-Woo Lee, Yufei Wang, Bolin Li, Guanshui Xie, Weijie Zhou, Changjing Xu, Hu Dingqin, Haihui Cai, Qing Lian, Longbin Qiu, Guangye Zhang, Mingwei An, Yang Wang, Bumjoon Kim, Xugang Guo, Bin Liu
High-performance organic solar cells (OSCs) demand precise control over the active layer morphology, as it greatly influences exciton dissociation and charge transport. Solid additives offer a powerful strategy for improved...
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DOI: 10.1039/D5EE01977J, PaperZhicheng Zhong, Sergio Gámez-Valenzuela, Jin-Woo Lee, Yufei Wang, Bolin Li, Guanshui Xie, Weijie Zhou, Changjing Xu, Hu Dingqin, Haihui Cai, Qing Lian, Longbin Qiu, Guangye Zhang, Mingwei An, Yang Wang, Bumjoon Kim, Xugang Guo, Bin Liu
High-performance organic solar cells (OSCs) demand precise control over the active layer morphology, as it greatly influences exciton dissociation and charge transport. Solid additives offer a powerful strategy for improved...
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Nanoplex-driven energy storage in relaxor antiferroelectrics
Energy Environ. Sci., 2025, Advance Article
DOI: 10.1039/D5EE02541A, PaperSimin Wang, Ke Xu, Guanglong Ge, Faqiang Zhang, Wangfeng Bai, Fei Yan, Jin Qian, Luomeng Tang, Yang Liu, Chao Sun, Zhongbin Pan, Bo Shen, Zhifu Liu, Houbing Huang, Jiwei Zhai
A novel nanoplex-driven architecture was constructed that integrated short-range ordered antiferroelectric nanodomains with highly disordered relaxor ferroelectrics.
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DOI: 10.1039/D5EE02541A, PaperSimin Wang, Ke Xu, Guanglong Ge, Faqiang Zhang, Wangfeng Bai, Fei Yan, Jin Qian, Luomeng Tang, Yang Liu, Chao Sun, Zhongbin Pan, Bo Shen, Zhifu Liu, Houbing Huang, Jiwei Zhai
A novel nanoplex-driven architecture was constructed that integrated short-range ordered antiferroelectric nanodomains with highly disordered relaxor ferroelectrics.
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Scalable Mechanochemical Synthesis of High-quality Prussian Blue Analogues for High-Energy and Durable Potassium-Ion Batteries
Energy Environ. Sci., 2025, Accepted Manuscript
DOI: 10.1039/D5EE01702E, PaperXunan Wang, Chongwei Gao, Shuhua Zhang, Jiantao Li, Jiali Wang, Shengdong Lin, Sungsik Lee, Feiyu Kang, Dengyun Zhai
Prussian blue analogues (PBAs) are recognized as promising cathode materials for potassium-ion batteries (PIBs), particularly the low-cost and high-energy K2Mn[Fe(CN)6](KMnF). However, conventional solution-based synthesis inevitably introduces [Fe(CN)6]4- defects and lattice...
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DOI: 10.1039/D5EE01702E, PaperXunan Wang, Chongwei Gao, Shuhua Zhang, Jiantao Li, Jiali Wang, Shengdong Lin, Sungsik Lee, Feiyu Kang, Dengyun Zhai
Prussian blue analogues (PBAs) are recognized as promising cathode materials for potassium-ion batteries (PIBs), particularly the low-cost and high-energy K2Mn[Fe(CN)6](KMnF). However, conventional solution-based synthesis inevitably introduces [Fe(CN)6]4- defects and lattice...
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Anchoring Ligand Engineering Enables Highly Stable MA-Free Perovskite Solar Cells with a Minimal Voc Deficit of 0.32 V
Energy Environ. Sci., 2025, Accepted Manuscript
DOI: 10.1039/D5EE03162A, Paper Open Access   This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.Chaohui Li, Andrej Vincze, Hyoungwon Park, Fabian Streller, Klaus Götz, Shudi Qiu, Jiwon Byun, Ying Shang, Zhangyu Yuan, Lirong Dong, Jingjing Tian, Zijian Peng, Chao Liu, Fu Yang, Yanxue Wang, Andreas Späth, Andres Osvet, Karen Forberich, Thomas Heumueller, Silke Christiansen, Marcus Halik, Rainer H. Fink, Tobias Unruh, Ning Li, Larry Lüer, Christoph J Brabec
Ligand engineering is an effective method to reduce defects in perovskite solar cells (PSCs) and to enhance efficiency. Likewise, enhancing device stability through ligand engineering is currently emerging as a...
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DOI: 10.1039/D5EE03162A, Paper Open Access   This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.Chaohui Li, Andrej Vincze, Hyoungwon Park, Fabian Streller, Klaus Götz, Shudi Qiu, Jiwon Byun, Ying Shang, Zhangyu Yuan, Lirong Dong, Jingjing Tian, Zijian Peng, Chao Liu, Fu Yang, Yanxue Wang, Andreas Späth, Andres Osvet, Karen Forberich, Thomas Heumueller, Silke Christiansen, Marcus Halik, Rainer H. Fink, Tobias Unruh, Ning Li, Larry Lüer, Christoph J Brabec
Ligand engineering is an effective method to reduce defects in perovskite solar cells (PSCs) and to enhance efficiency. Likewise, enhancing device stability through ligand engineering is currently emerging as a...
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Balancing Solvation: Stabilizing Lithium Metal Batteries via Optimized Cosolvents in Ionic-liquid Electrolytes
Energy Environ. Sci., 2025, Accepted Manuscript
DOI: 10.1039/D5EE01515D, Paper Open Access   This article is licensed under a Creative Commons Attribution-NonCommercial 3.0 Unported Licence.Xinlin Li, Xianyang Wu, Seoung-Bum Son, Jorge M Seminario, Perla B Balbuena, Anderson Arboleda, Jiyu Cai, Matthew Li, Ziyuan Lyu, Dominic Bresser, Rachid Amine, Chi Cheung Su, Khalil Amine
In this study, we examined three co-solvents with distinct solvation capabilities for ionic-liquid-based electrolytes, 1-methyl-1-propyl pyrrolidinium bis(fluorosulfonyl)imide (Py13FSI). Among them, we demonstrate that 1,1,1-trifluoro-2-(2-(2-(2,2,2-trifluoroethoxy)ethoxy)ethoxy)ethane (FDG), notably enhances the cycle life...
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DOI: 10.1039/D5EE01515D, Paper Open Access   This article is licensed under a Creative Commons Attribution-NonCommercial 3.0 Unported Licence.Xinlin Li, Xianyang Wu, Seoung-Bum Son, Jorge M Seminario, Perla B Balbuena, Anderson Arboleda, Jiyu Cai, Matthew Li, Ziyuan Lyu, Dominic Bresser, Rachid Amine, Chi Cheung Su, Khalil Amine
In this study, we examined three co-solvents with distinct solvation capabilities for ionic-liquid-based electrolytes, 1-methyl-1-propyl pyrrolidinium bis(fluorosulfonyl)imide (Py13FSI). Among them, we demonstrate that 1,1,1-trifluoro-2-(2-(2-(2,2,2-trifluoroethoxy)ethoxy)ethoxy)ethane (FDG), notably enhances the cycle life...
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