RSC - Energy Environ. Sci. latest articles
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Metallurgical refractory lining-guided inorganic binder for stable lithium storage in silicon microparticle anodes
Energy Environ. Sci., 2025, Accepted Manuscript
DOI: 10.1039/D5EE03194J, CommunicationJinwei Zhou, Siyao Wu, Yang Li, Qihou Li, Feixiang Wu
Silicon is a promising anode material for next-generation lithium-ion batteries (LIBs), offering a significantly higher theoretical capacity than graphite. While nano-silicon excels, its high cost limits practicality, making silicon microparticles...
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DOI: 10.1039/D5EE03194J, CommunicationJinwei Zhou, Siyao Wu, Yang Li, Qihou Li, Feixiang Wu
Silicon is a promising anode material for next-generation lithium-ion batteries (LIBs), offering a significantly higher theoretical capacity than graphite. While nano-silicon excels, its high cost limits practicality, making silicon microparticles...
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Methane Photolysis to Clean Hydrogen and Carbon Nanotubes
Energy Environ. Sci., 2025, Accepted Manuscript
DOI: 10.1039/D5EE02120K, Paper Open Access   This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.Geoffrey A. Ozin, Abdelaziz Gouda, Nazir Kherani, Nhat Truong Nguyen, Juan Manuel Restrepo Florez, Mohini M. Sain, Camilo Viasus, Jessica Ye, Abhinav Mohan, Otavio Augusto Titton Dias, Vijay K Tomer, Andrew Wang, Tamlyn Slocombe, Alan Aspuru-Guzik, Jiabao Shen, Mohamad Hmadeh
The transition to sustainable hydrogen production is critical to decarbonizing the global energy system and reducing reliance on carbon-intensive methods such as steam methane reforming (SMR). Methane pyrolysis has emerged...
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DOI: 10.1039/D5EE02120K, Paper Open Access   This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.Geoffrey A. Ozin, Abdelaziz Gouda, Nazir Kherani, Nhat Truong Nguyen, Juan Manuel Restrepo Florez, Mohini M. Sain, Camilo Viasus, Jessica Ye, Abhinav Mohan, Otavio Augusto Titton Dias, Vijay K Tomer, Andrew Wang, Tamlyn Slocombe, Alan Aspuru-Guzik, Jiabao Shen, Mohamad Hmadeh
The transition to sustainable hydrogen production is critical to decarbonizing the global energy system and reducing reliance on carbon-intensive methods such as steam methane reforming (SMR). Methane pyrolysis has emerged...
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Unveiling the Single-Solvent Vacuum-Flash Process for High-Efficiency Perovskite Solar Cells
Energy Environ. Sci., 2025, Accepted Manuscript
DOI: 10.1039/D5EE05421D, PaperHuanyu Zhang, Yige Peng, Yurou Zhang, Yi Ji, Zewu Feng, Hailong Huang, Yanbo Wang, Yansen Guo, Chenghao Ge, Xin Li, Xueqi Wu, Yitong Liu, Chaopeng Huang, Jingsong Sun, Xiaohong Zhang, Jun Peng
High-crystallinity perovskite films with low trap density are a prerequisite for realizing high-performance perovskite solar cells (PSCs). Here, we present a straightforward single-solvent vacuum-flash (SSVF) method for fabricating high-quality perovskite...
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DOI: 10.1039/D5EE05421D, PaperHuanyu Zhang, Yige Peng, Yurou Zhang, Yi Ji, Zewu Feng, Hailong Huang, Yanbo Wang, Yansen Guo, Chenghao Ge, Xin Li, Xueqi Wu, Yitong Liu, Chaopeng Huang, Jingsong Sun, Xiaohong Zhang, Jun Peng
High-crystallinity perovskite films with low trap density are a prerequisite for realizing high-performance perovskite solar cells (PSCs). Here, we present a straightforward single-solvent vacuum-flash (SSVF) method for fabricating high-quality perovskite...
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Sodium-compensating electrolyte additive stabilizes interfaces for highly reversible anode-free sodium batteries
Energy Environ. Sci., 2025, Accepted Manuscript
DOI: 10.1039/D5EE04804D, PaperChunlin Xie, Shengfang Liu, Jin Wang, Xianghui Meng, Shuyi Yu, Jiaming Zhang, Haijun Peng, Dan Sun, Yougen Tang, Hai-Yan Wang
Anode-free sodium batteries (AFSBs) offer superior cost, energy density, and manufacturing advantages over sodium-ion batteries (SIBs) by eliminating the conventional anode. However, their development is fundamentally hindered by dead sodium...
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DOI: 10.1039/D5EE04804D, PaperChunlin Xie, Shengfang Liu, Jin Wang, Xianghui Meng, Shuyi Yu, Jiaming Zhang, Haijun Peng, Dan Sun, Yougen Tang, Hai-Yan Wang
Anode-free sodium batteries (AFSBs) offer superior cost, energy density, and manufacturing advantages over sodium-ion batteries (SIBs) by eliminating the conventional anode. However, their development is fundamentally hindered by dead sodium...
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Hydration Equilibrium-controlled Cation-Anion Coordination Competition for Precise Recovery of All Valuable Metals from Spent Lithium-ion Batteries
Energy Environ. Sci., 2025, Accepted Manuscript
DOI: 10.1039/D5EE05276A, PaperMingqiang Cheng, Juanjian Ru, Shukai Miao, Yixin Hua, Qibo Zhang, Cunying Xu, Zhipeng Zhou, Ding WANG, Wenchao Zhang, Jiexi Wang, Zaiping Guo
The selective recovery of metals from spent lithium-ion batteries (LIBs), particularly from Ni-based ternary (NCM) cathode materials, is a significant challenge due to their complex elemental composition. Herein, we present...
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DOI: 10.1039/D5EE05276A, PaperMingqiang Cheng, Juanjian Ru, Shukai Miao, Yixin Hua, Qibo Zhang, Cunying Xu, Zhipeng Zhou, Ding WANG, Wenchao Zhang, Jiexi Wang, Zaiping Guo
The selective recovery of metals from spent lithium-ion batteries (LIBs), particularly from Ni-based ternary (NCM) cathode materials, is a significant challenge due to their complex elemental composition. Herein, we present...
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Boron–halide interactions for crystallization regulation of a 1.68 eV wide-bandgap perovskite prepared via a two-step method
Energy Environ. Sci., 2025, Advance Article
DOI: 10.1039/D5EE03984C, Paper Open Access   This article is licensed under a Creative Commons Attribution-NonCommercial 3.0 Unported Licence.Shizi Luo, Daxiong Liu, Xiang Deng, Zhuoneng Bi, Shuguang Cao, Tongjun Zheng, Liyao Xiong, Hao Li, Ning Li, Lavrenty G. Gutsev, Nikita A. Emelianov, Victoria V. Ozerova, Nikita A. Slesarenko, Alexander F. Shestakov, Sergey M. Aldoshin, Gennady L. Gutsev, Pavel A. Troshin, Bochuan Yang, Zhibo Zhao, Xueqing Xu
Leveraging tris(pentafluorophenyl)borane (BCF) to regulate crystallization of perovskite by the boron–halogen and hydrogen bonding effects enabled a PCE of 23.49% and 31.12% at 1.68 eV for single-junction PSCs and perovskite/Si TSCs, respectively.
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DOI: 10.1039/D5EE03984C, Paper Open Access   This article is licensed under a Creative Commons Attribution-NonCommercial 3.0 Unported Licence.Shizi Luo, Daxiong Liu, Xiang Deng, Zhuoneng Bi, Shuguang Cao, Tongjun Zheng, Liyao Xiong, Hao Li, Ning Li, Lavrenty G. Gutsev, Nikita A. Emelianov, Victoria V. Ozerova, Nikita A. Slesarenko, Alexander F. Shestakov, Sergey M. Aldoshin, Gennady L. Gutsev, Pavel A. Troshin, Bochuan Yang, Zhibo Zhao, Xueqing Xu
Leveraging tris(pentafluorophenyl)borane (BCF) to regulate crystallization of perovskite by the boron–halogen and hydrogen bonding effects enabled a PCE of 23.49% and 31.12% at 1.68 eV for single-junction PSCs and perovskite/Si TSCs, respectively.
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Cathode Passivation Suppression Enables Ultrastable Industry-Leading Alkaline Water Electrolysis at Hundred-Ampere Currents
Energy Environ. Sci., 2025, Accepted Manuscript
DOI: 10.1039/D5EE04506A, PaperYang Wu, Zhenhui Kou, Nengji Liu, Senlin Chu, Bin Yang, Zhongjian Li, Juan Shang, Fei Song, Qinghua Zhang, Peng Liao, Youxiao Chen, Lecheng Lei, Yang Hou
Industry-leading alkaline water electrolysis (AWE) remains limited to low current densities (<0.3 A cm-2) due to cathodic oxidation-induced passivation of commercial Raney Ni cathodes under operation. This generates interfacial...
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DOI: 10.1039/D5EE04506A, PaperYang Wu, Zhenhui Kou, Nengji Liu, Senlin Chu, Bin Yang, Zhongjian Li, Juan Shang, Fei Song, Qinghua Zhang, Peng Liao, Youxiao Chen, Lecheng Lei, Yang Hou
Industry-leading alkaline water electrolysis (AWE) remains limited to low current densities (<0.3 A cm-2) due to cathodic oxidation-induced passivation of commercial Raney Ni cathodes under operation. This generates interfacial...
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A sustained-release strategy of fluorinated solvents enables highly safe lithium metal batteries
Energy Environ. Sci., 2025, Advance Article
DOI: 10.1039/D5EE03640B, PaperZhimeng Sheng, Xiaoyu Guo, Rong Gu, Shengtao Xu, Yizheng Ma, Jiayao Shan, Zhangyue Wei, Hongyu Shi, Shuaiqi Gong, Jinting Xu, Yan Zhang, Sheng Zhu, Guodong Qi, Yulin Min
This study proposes a fluorinated solvent sustained-release strategy, which enables the gradual release of fluorinated solvents during thermal runaway.
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DOI: 10.1039/D5EE03640B, PaperZhimeng Sheng, Xiaoyu Guo, Rong Gu, Shengtao Xu, Yizheng Ma, Jiayao Shan, Zhangyue Wei, Hongyu Shi, Shuaiqi Gong, Jinting Xu, Yan Zhang, Sheng Zhu, Guodong Qi, Yulin Min
This study proposes a fluorinated solvent sustained-release strategy, which enables the gradual release of fluorinated solvents during thermal runaway.
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Ultra-Low-Loading RuW Nanoclusters Coupled with W Single Atoms for Efficient Anion Exchange Membrane Fuel Cells
Energy Environ. Sci., 2025, Accepted Manuscript
DOI: 10.1039/D5EE04114G, PaperQingping Yu, Rong Liu, Licheng Wei, Zhenying Zheng, Lifeng Zhang, Hu Yang, Qingyu Kong, Jihao Zhang, Zhiwei Hu, Qilei Song, Xiaoping Gao, Nanjun Chen, Xiaoqing Huang
Cost-effective Ru holds promise to tackle the sluggish hydrogen oxidation reaction (HOR) kinetic under alkaline conditions, which has emerged as an appealing alternative to Pt and Pt-Ru. However, developing Ru-type...
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DOI: 10.1039/D5EE04114G, PaperQingping Yu, Rong Liu, Licheng Wei, Zhenying Zheng, Lifeng Zhang, Hu Yang, Qingyu Kong, Jihao Zhang, Zhiwei Hu, Qilei Song, Xiaoping Gao, Nanjun Chen, Xiaoqing Huang
Cost-effective Ru holds promise to tackle the sluggish hydrogen oxidation reaction (HOR) kinetic under alkaline conditions, which has emerged as an appealing alternative to Pt and Pt-Ru. However, developing Ru-type...
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Interface Molecular Orientation Engineering Induced Field Reversal for Efficient Inverted Perovskite Solar Cells
Energy Environ. Sci., 2025, Accepted Manuscript
DOI: 10.1039/D5EE02667A, PaperSuhao Yan, Bo Zhang, Wenguang Zhang, Kun Chen, Zijuan He, Yang Sun, Haipeng Yin, Zi Ouyang, Xin Li, Bo Xiao
Inverted perovskite solar cells (PSCs) continue to suffer from severe non-radiative recombination and low carrier transportation at the perovskite/C60 interface. Traditional passivation layers typically improve the device's open-circuit voltage while...
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DOI: 10.1039/D5EE02667A, PaperSuhao Yan, Bo Zhang, Wenguang Zhang, Kun Chen, Zijuan He, Yang Sun, Haipeng Yin, Zi Ouyang, Xin Li, Bo Xiao
Inverted perovskite solar cells (PSCs) continue to suffer from severe non-radiative recombination and low carrier transportation at the perovskite/C60 interface. Traditional passivation layers typically improve the device's open-circuit voltage while...
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Dual modulation of coordination asymmetry and curvature unlocks record-level Zn-air battery performance with Fe-N-C single-atom catalysts
Energy Environ. Sci., 2025, Accepted Manuscript
DOI: 10.1039/D5EE04648C, PaperQichen Wang, Lulu Lyu, Nannan Han, Bingxian Chu, Chunyan Shang, Ziyi Wang, Hetong Pan, Dongjun Lee, Wang Zhang, Junfeng Zhang, Zhipeng Li, Wei Huang, Yong-Mook Kang
The coordination environment of single-atom catalysts (SACs) plays a pivotal role in determining their electronic structure and catalytic performance. Conventional planar Fe-N4 motifs, however, often bind oxygen intermediates too strongly,...
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DOI: 10.1039/D5EE04648C, PaperQichen Wang, Lulu Lyu, Nannan Han, Bingxian Chu, Chunyan Shang, Ziyi Wang, Hetong Pan, Dongjun Lee, Wang Zhang, Junfeng Zhang, Zhipeng Li, Wei Huang, Yong-Mook Kang
The coordination environment of single-atom catalysts (SACs) plays a pivotal role in determining their electronic structure and catalytic performance. Conventional planar Fe-N4 motifs, however, often bind oxygen intermediates too strongly,...
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Surface-Tension Induced High Packing Density Carbon Nanoribbons Film with Ultrahigh Volumetric Capacitance
Energy Environ. Sci., 2025, Accepted Manuscript
DOI: 10.1039/D5EE02047F, PaperXiao Jun Shi, Huanwen Wang, Taoqiu Zhang, Tong Xue, Haiyong He, Hong Jin Fan
For ultrafast-response supercapacitors, it is very challenging for typical porous carbon electrodes to exhibit both high volumetric (Cv) and areal (Ca) capacitances, especially under high rates, due to inefficient pore...
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DOI: 10.1039/D5EE02047F, PaperXiao Jun Shi, Huanwen Wang, Taoqiu Zhang, Tong Xue, Haiyong He, Hong Jin Fan
For ultrafast-response supercapacitors, it is very challenging for typical porous carbon electrodes to exhibit both high volumetric (Cv) and areal (Ca) capacitances, especially under high rates, due to inefficient pore...
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Primacy of lattice distortion over strain in platinum fuel cell nanoalloy catalysts
Energy Environ. Sci., 2025, Accepted Manuscript
DOI: 10.1039/D5EE04563K, PaperAmir Gasmi, Meryem Ennaji, Ashwin Thirumalai Shekhar, Rémi Bacabe, Morgane Stodel, Frédéric Lecoeur, Marc Dupont, Camille Roiron, Raphael Chattot, Carlos Augusto Augusto Campos Roldán, Valentin Vinci, Marta Mirolo, Jakub Drnec, Deborah J. Jones
Alloying platinum with early or late transition metals enhances its intrinsic activity toward the oxygen reduction reaction for proton exchange membrane fuel cells (PEMFCs), according to strain and ligand effects....
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DOI: 10.1039/D5EE04563K, PaperAmir Gasmi, Meryem Ennaji, Ashwin Thirumalai Shekhar, Rémi Bacabe, Morgane Stodel, Frédéric Lecoeur, Marc Dupont, Camille Roiron, Raphael Chattot, Carlos Augusto Augusto Campos Roldán, Valentin Vinci, Marta Mirolo, Jakub Drnec, Deborah J. Jones
Alloying platinum with early or late transition metals enhances its intrinsic activity toward the oxygen reduction reaction for proton exchange membrane fuel cells (PEMFCs), according to strain and ligand effects....
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Robust Interfaces via Synergistic Cation-Anion Manipulation for Highly Efficient and Stable Inverted Perovskite Solar Cells
Energy Environ. Sci., 2025, Accepted Manuscript
DOI: 10.1039/D5EE04111B, PaperHaoze Lu, Yang Yang, Ruihao Chen, Zhiyuan Dai, Yuming Liu, Shuyuan Wan, Jinhan Sun, Dilnaz Kadyrma, Anar Dosmukhambetovab, Yerzhan Mukhametkarimov, Zhe Liu, Hongqiang Wang
Ionic defect sites at planar photovoltaic interfaces cause usually the degradation of perovskite solar cells (PSCs), where uncoordinated ions and consequent instable counterions are the intrinsic reasons behind the interfacial...
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DOI: 10.1039/D5EE04111B, PaperHaoze Lu, Yang Yang, Ruihao Chen, Zhiyuan Dai, Yuming Liu, Shuyuan Wan, Jinhan Sun, Dilnaz Kadyrma, Anar Dosmukhambetovab, Yerzhan Mukhametkarimov, Zhe Liu, Hongqiang Wang
Ionic defect sites at planar photovoltaic interfaces cause usually the degradation of perovskite solar cells (PSCs), where uncoordinated ions and consequent instable counterions are the intrinsic reasons behind the interfacial...
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Ion Exchange-Induced LixMgyBOz Coating Synergized with Reinforced Bulk Doping Enables Fast-Charging Long-Cycling High-Voltage LiCoO2
Energy Environ. Sci., 2025, Accepted Manuscript
DOI: 10.1039/D5EE04240B, PaperTing Wang, Yuqi Zhou, Jiaqi Huang, Fangzhou Zhao, Wanglai Cen, Lanlu Lu, Yifei Dang, Kecheng Cao, Yan Meng, Yongzhi Zhang, Dan Xiao
Under high-voltage conditions (>4.5 V vs. Li+ /Li), the practical application of LiCoO2 (LCO) is severely limited by irreversible structural degradation and interfacial instability. Herein, we propose a computationally guided...
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DOI: 10.1039/D5EE04240B, PaperTing Wang, Yuqi Zhou, Jiaqi Huang, Fangzhou Zhao, Wanglai Cen, Lanlu Lu, Yifei Dang, Kecheng Cao, Yan Meng, Yongzhi Zhang, Dan Xiao
Under high-voltage conditions (>4.5 V vs. Li+ /Li), the practical application of LiCoO2 (LCO) is severely limited by irreversible structural degradation and interfacial instability. Herein, we propose a computationally guided...
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Regioisomerism-Guided Interfacial Design toward Stable Zinc Metal Anodes
Energy Environ. Sci., 2025, Accepted Manuscript
DOI: 10.1039/D5EE04705F, PaperJiaming Li, Hanhao Liang, Nan Li, Junyi Han, Jiaqi Li, Hedong Gu, Shaoyu Zhang, Jianhang Huang, Zhanhong Yang, Yongyao Xia
The interfacial instability of zinc metal anodes is one of the key obstacles limiting the practical commercialization of aqueous zinc-ion batteries (AZIBs). In recent years, the introduction of small organic...
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DOI: 10.1039/D5EE04705F, PaperJiaming Li, Hanhao Liang, Nan Li, Junyi Han, Jiaqi Li, Hedong Gu, Shaoyu Zhang, Jianhang Huang, Zhanhong Yang, Yongyao Xia
The interfacial instability of zinc metal anodes is one of the key obstacles limiting the practical commercialization of aqueous zinc-ion batteries (AZIBs). In recent years, the introduction of small organic...
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Diagnosing mechanisms to mitigate anion exchange ionomer degradation during impure water electrolysis
Energy Environ. Sci., 2025, Advance Article
DOI: 10.1039/D5EE03891J, PaperIsabela Rios Amador, Ryan T. Hannagan, Allen Qiang, Sang-Won Lee, Nhi Thi Thu Tran, Kyra M. K. Yap, Ashton M. Aleman, Daniela H. Marin, Milenia Rojas Mendoza, Michaela Burke Stevens, Thomas F. Jaramillo, Adam C. Nielander
We analyzed chemical and electrochemical degradation products and pathways of PiperION under oxidizing conditions in saline electrolyte to gain understanding toward ionomer degradation under impure water electrolysis.
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DOI: 10.1039/D5EE03891J, PaperIsabela Rios Amador, Ryan T. Hannagan, Allen Qiang, Sang-Won Lee, Nhi Thi Thu Tran, Kyra M. K. Yap, Ashton M. Aleman, Daniela H. Marin, Milenia Rojas Mendoza, Michaela Burke Stevens, Thomas F. Jaramillo, Adam C. Nielander
We analyzed chemical and electrochemical degradation products and pathways of PiperION under oxidizing conditions in saline electrolyte to gain understanding toward ionomer degradation under impure water electrolysis.
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Molecularly guided buried-interface regulation for efficient and stable inverted perovskite solar cells
Energy Environ. Sci., 2025, Accepted Manuscript
DOI: 10.1039/D5EE05094D, PaperQuanzhou Li, Min Wang, Liang Li
Inverted perovskite solar cells (IPSCs) are among the most promising candidates for scalable photovoltaics, yet their buried interfaces remain a critical bottleneck that limits efficiency and long-term stability. In particular,...
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DOI: 10.1039/D5EE05094D, PaperQuanzhou Li, Min Wang, Liang Li
Inverted perovskite solar cells (IPSCs) are among the most promising candidates for scalable photovoltaics, yet their buried interfaces remain a critical bottleneck that limits efficiency and long-term stability. In particular,...
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Toward a Sustainable Energy Future Using Ammonia as an Energy Carrier: Global Supply Chain Cost and Greenhouse Gas Emissions
Energy Environ. Sci., 2025, Accepted Manuscript
DOI: 10.1039/D5EE05571G, Paper Open Access   This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.Woojae Shin, Haoxiang Lai, Gasim Ibrahim, Guiyan Zang
A comprehensive techno-economic and environmental assessment database for global ammonia supply chains was developed across 63 countries, assessing diverse production technologies (gray, blue, yellow, pink, green) and downstream logistics by...
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DOI: 10.1039/D5EE05571G, Paper Open Access   This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.Woojae Shin, Haoxiang Lai, Gasim Ibrahim, Guiyan Zang
A comprehensive techno-economic and environmental assessment database for global ammonia supply chains was developed across 63 countries, assessing diverse production technologies (gray, blue, yellow, pink, green) and downstream logistics by...
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Unveiling the role of halide mixing on crystallization kinetics and charge transfer mechanisms in wide-bandgap organic-inorganic halide perovskites
Energy Environ. Sci., 2025, Accepted Manuscript
DOI: 10.1039/D5EE05540G, Paper Open Access   This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.Nian Li, Shambhavi Pratap, Renjun Guo, Zirui He, Suzhe Liang, Xiangkun Jia, Mohammad Gholipoor, Finn Babbe, Nicola S Barchi, Jonathan L. Slack, Nobumichi Tamura, Liang Qiao, Carolin M. Sutter-Fella, Peter Müller-Buschbaum
Despite many efforts to increase the photovoltaic performances of wide-bandgap (WBG, with Br content above 20%) perovskite solar cells based on bromine-iodine (Br-I) mixed-halide perovskites, understanding the crystallization kinetics of...
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DOI: 10.1039/D5EE05540G, Paper Open Access   This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.Nian Li, Shambhavi Pratap, Renjun Guo, Zirui He, Suzhe Liang, Xiangkun Jia, Mohammad Gholipoor, Finn Babbe, Nicola S Barchi, Jonathan L. Slack, Nobumichi Tamura, Liang Qiao, Carolin M. Sutter-Fella, Peter Müller-Buschbaum
Despite many efforts to increase the photovoltaic performances of wide-bandgap (WBG, with Br content above 20%) perovskite solar cells based on bromine-iodine (Br-I) mixed-halide perovskites, understanding the crystallization kinetics of...
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