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Machine learning-assisted benign transformation of three zinc states in zinc ion batteries
Energy Environ. Sci., 2025, Advance Article
DOI: 10.1039/D5EE00650C, Paper Open Access   This article is licensed under a Creative Commons Attribution-NonCommercial 3.0 Unported Licence.Jianbo Dong, Guolang Zhou, Wenhao Ding, Jiayi Ji, Qing Wang, Tianshi Wang, Lili Zhang, Xiuyang Zou, Jingzhou Yin, Edison Huixiang Ang
A machine-learning-designed cerium-iron MOF layer enhances Zn anode stability, achieving over 4300 hours at 1 mA cm−2 and 99.8% coulombic efficiency over 1400 cycles at 2 mA cm−2, providing a cost-effective protective strategy.
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DOI: 10.1039/D5EE00650C, Paper Open Access   This article is licensed under a Creative Commons Attribution-NonCommercial 3.0 Unported Licence.Jianbo Dong, Guolang Zhou, Wenhao Ding, Jiayi Ji, Qing Wang, Tianshi Wang, Lili Zhang, Xiuyang Zou, Jingzhou Yin, Edison Huixiang Ang
A machine-learning-designed cerium-iron MOF layer enhances Zn anode stability, achieving over 4300 hours at 1 mA cm−2 and 99.8% coulombic efficiency over 1400 cycles at 2 mA cm−2, providing a cost-effective protective strategy.
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One-Stone-Two-Birds: Over 26% Efficiency in Perovskite Solar Cells via Synergistic Crystallization & Interface Regulation
Energy Environ. Sci., 2025, Accepted Manuscript
DOI: 10.1039/D5EE00189G, PaperBoxin Jiao, Liguo Tan, Yiran Ye, Ningyu Ren, Minghao Li, Hang Li, Xiaoyi Li, Chenyi Yi
Organic-inorganic hybrid perovskites have emerged as promising photovoltaic materials due to their excellent photoelectronic properties and low-cost fabrication techniques. However, the performance and stability of perovskite solar cells (PSCs) are...
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DOI: 10.1039/D5EE00189G, PaperBoxin Jiao, Liguo Tan, Yiran Ye, Ningyu Ren, Minghao Li, Hang Li, Xiaoyi Li, Chenyi Yi
Organic-inorganic hybrid perovskites have emerged as promising photovoltaic materials due to their excellent photoelectronic properties and low-cost fabrication techniques. However, the performance and stability of perovskite solar cells (PSCs) are...
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Sustainable Protection of Natural Liquid Enables Ultra-Stable Inverted Perovskite Solar Cells via Allylic Disulfide Rearrangement
Energy Environ. Sci., 2025, Accepted Manuscript
DOI: 10.1039/D5EE00458F, PaperYang Yang, Shuyuan Wan, Hang Wei, Lijun Yang, Zhiyuan Dai, Haoze Lu, Zhe Liu, Bo Chen, Ruihao Chen, Hongqiang Wang
Perovskite solar cells (PSCs) suffer from instability under prolonged exposure to light, moisture, and heat, primarily due to uncoordinated ionic defects. Current strategies primarily focus on using solid-state molecules to...
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DOI: 10.1039/D5EE00458F, PaperYang Yang, Shuyuan Wan, Hang Wei, Lijun Yang, Zhiyuan Dai, Haoze Lu, Zhe Liu, Bo Chen, Ruihao Chen, Hongqiang Wang
Perovskite solar cells (PSCs) suffer from instability under prolonged exposure to light, moisture, and heat, primarily due to uncoordinated ionic defects. Current strategies primarily focus on using solid-state molecules to...
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Internal and External Cultivation: Unleashing the Potential of Photogenerated Carrier Dynamics Behaviors to Boost Photocatalytic CO2 Hydrogenation
Energy Environ. Sci., 2025, Accepted Manuscript
DOI: 10.1039/D5EE00605H, PaperYuhao Guo, Qinhui Guan, Xingjuan Li, Mengjun Zhao, Na Li, Zizhong Zhang, Gui-qiang Fei, Tingjiang Yan
In heterogeneous photocatalysis, the dynamics of charge carriers holds particular significance for comprehending the underlying catalytic mechanism and designing highly efficient photocatalysts. The current technological challenge lies in how to...
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DOI: 10.1039/D5EE00605H, PaperYuhao Guo, Qinhui Guan, Xingjuan Li, Mengjun Zhao, Na Li, Zizhong Zhang, Gui-qiang Fei, Tingjiang Yan
In heterogeneous photocatalysis, the dynamics of charge carriers holds particular significance for comprehending the underlying catalytic mechanism and designing highly efficient photocatalysts. The current technological challenge lies in how to...
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Achieving a higher lithium density in anode surpassing that of pure metallic lithium for high-energy-density batteries
Energy Environ. Sci., 2025, Accepted Manuscript
DOI: 10.1039/D4EE05289G, PaperXiancheng Wang, Bao Zhang, Zihe Chen, Shiyu Liu, Wenyu Wang, Shuibin Tu, Renming Zhan, Li Wang, Yongming Sun
The low-density, high-porosity lithium (Li) plating layer at the anode is one of the principal determinants of the overall volumetric expansion in rechargeable high-energy-density Li metal batteries, which account for...
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DOI: 10.1039/D4EE05289G, PaperXiancheng Wang, Bao Zhang, Zihe Chen, Shiyu Liu, Wenyu Wang, Shuibin Tu, Renming Zhan, Li Wang, Yongming Sun
The low-density, high-porosity lithium (Li) plating layer at the anode is one of the principal determinants of the overall volumetric expansion in rechargeable high-energy-density Li metal batteries, which account for...
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Ligand effects enhancing low-temperature oxygen reduction kinetics in neutral conditions
Energy Environ. Sci., 2025, Accepted Manuscript
DOI: 10.1039/D5EE01407G, PaperYongjian Zhao, Murong Huang, Yongshuai Kang, Yong Fang, Tianyou Zhao, Hu Wang, Jiayi Ou, Jiajun Liu, Meixi Zhong, Tao Wang, Xianhu Sun, Chenyang Zhao, Dan Wang
The sluggish oxygen reduction kinetics, resulting from ineffective O2 activation and hydrogenation, has been hindering the performance improvement of self-breathing zinc-air batteries (ZABs), especially in a hostile environment under low...
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DOI: 10.1039/D5EE01407G, PaperYongjian Zhao, Murong Huang, Yongshuai Kang, Yong Fang, Tianyou Zhao, Hu Wang, Jiayi Ou, Jiajun Liu, Meixi Zhong, Tao Wang, Xianhu Sun, Chenyang Zhao, Dan Wang
The sluggish oxygen reduction kinetics, resulting from ineffective O2 activation and hydrogenation, has been hindering the performance improvement of self-breathing zinc-air batteries (ZABs), especially in a hostile environment under low...
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Polyphosphonitrile Derivative-Based Gel Electrolytes for All-Climate Zinc Metal Batteries Operating from −70 oC to +80 oC
Energy Environ. Sci., 2025, Accepted Manuscript
DOI: 10.1039/D5EE01478F, PaperRan Han, Yuefeng Meng, Xin Zhao, Yao Wang, Mingkun Tang, Yichen Ding, Baohua Li, Dong Zhou, Feiyu Kang
The high freezing point and poor anode stability of traditional aqueous electrolytes strongly hamper the cyclability and working temperature range of zinc (Zn) metal batteries (ZMBs). Herein, we demonstrate a...
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DOI: 10.1039/D5EE01478F, PaperRan Han, Yuefeng Meng, Xin Zhao, Yao Wang, Mingkun Tang, Yichen Ding, Baohua Li, Dong Zhou, Feiyu Kang
The high freezing point and poor anode stability of traditional aqueous electrolytes strongly hamper the cyclability and working temperature range of zinc (Zn) metal batteries (ZMBs). Herein, we demonstrate a...
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Fully evaporated interfacial layers for high-performance and batch-to-batch reproducible organic solar modules
Energy Environ. Sci., 2025, Accepted Manuscript
DOI: 10.1039/D5EE00014A, PaperZe Jin, Cheng Shen, Haotian Hu, Chengcheng Han, Yongqi Bai, Mengjin Yang, Quan Liu, Ziyi Ge
Significant advancements in research have been made in recent years, with single-junction organic solar cells achieving efficiencies exceeding 20%. However, scaling up laboratory prototypes to large-area commercial modules remains challenging...
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DOI: 10.1039/D5EE00014A, PaperZe Jin, Cheng Shen, Haotian Hu, Chengcheng Han, Yongqi Bai, Mengjin Yang, Quan Liu, Ziyi Ge
Significant advancements in research have been made in recent years, with single-junction organic solar cells achieving efficiencies exceeding 20%. However, scaling up laboratory prototypes to large-area commercial modules remains challenging...
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Tetragonal ZrO2 supported low-iridium catalyst activating oxygen spillover stabilized lattice oxygen for proton exchange membrane water electrolysis
Energy Environ. Sci., 2025, Accepted Manuscript
DOI: 10.1039/D5EE00544B, PaperSong Ru Fang, Hai Xiang Yang, Hao Yang Lin, Miaoyu Lin, Fangxin Mao, Hao Fan, Huai Qin Fu, Haiyang Yuan, Chenghua Sun, Peng Fei Liu, Huagui Yang
Mediating the trade-off between activity and durability at a low Ir loading is challengeable for acidic oxygen evolution reaction (OER) in proton exchange membrane (PEM) water electrolysis. Herein, we construct...
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DOI: 10.1039/D5EE00544B, PaperSong Ru Fang, Hai Xiang Yang, Hao Yang Lin, Miaoyu Lin, Fangxin Mao, Hao Fan, Huai Qin Fu, Haiyang Yuan, Chenghua Sun, Peng Fei Liu, Huagui Yang
Mediating the trade-off between activity and durability at a low Ir loading is challengeable for acidic oxygen evolution reaction (OER) in proton exchange membrane (PEM) water electrolysis. Herein, we construct...
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Modeling carbon-free energy conversion systems: enhanced hydrazine-assisted hydrogen production with dual-electric-field effect on needle-like Ru/CoP catalysts
Energy Environ. Sci., 2025, Advance Article
DOI: 10.1039/D4EE05691D, PaperKang Ji, Shiyu Wang, Shuyun Yao, Yingjie Ji, Guixi Wang, Weikun Ren, Jun Wang, Feike Zhang, Jiangzhou Xie, Zhiyu Yang, Yi-Ming Yan
The local electric field weakens the hydrogen-bond network and enhances H2O transport. The built-in electric field creates electron-deficient sites, improving the adsorption of N2H4. Finally, a self-powered zero-carbon energy system was built.
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DOI: 10.1039/D4EE05691D, PaperKang Ji, Shiyu Wang, Shuyun Yao, Yingjie Ji, Guixi Wang, Weikun Ren, Jun Wang, Feike Zhang, Jiangzhou Xie, Zhiyu Yang, Yi-Ming Yan
The local electric field weakens the hydrogen-bond network and enhances H2O transport. The built-in electric field creates electron-deficient sites, improving the adsorption of N2H4. Finally, a self-powered zero-carbon energy system was built.
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Synergy of phase and interface engineering of manganese difluoride enable high-efficiency potassium-ion batteries
Energy Environ. Sci., 2025, Accepted Manuscript
DOI: 10.1039/D5EE00499C, PaperXinru Sheng, Jiaying Liao, Zeyu Yuan, Yuhan Wang, Qiao Hu, Yichen Du, Xuefeng Wang, Xiaosi Zhou
Conversion-type materials are regarded as potential anodes for potassium-ion batteries, achieving high potassium storage capacity through conversion reactions to form K-rich compounds. However, the accompanying huge volume change often brings...
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DOI: 10.1039/D5EE00499C, PaperXinru Sheng, Jiaying Liao, Zeyu Yuan, Yuhan Wang, Qiao Hu, Yichen Du, Xuefeng Wang, Xiaosi Zhou
Conversion-type materials are regarded as potential anodes for potassium-ion batteries, achieving high potassium storage capacity through conversion reactions to form K-rich compounds. However, the accompanying huge volume change often brings...
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Compacting surface charge Layer for efficient charge transfer toward stable Zn anode
Energy Environ. Sci., 2025, Accepted Manuscript
DOI: 10.1039/D5EE01092F, PaperSinan Zheng, Yang Wang, Bin Luo, Kun Zhang, Leilei Sun, Zhean Bao, Guosheng Duan, Dinghao Chen, Hanwei Hu, Jingyun Huang, Zhizhen Ye
The dynamic reconstruction of electric double layers (EDLs) holds the key to stabilizing aqueous Zn metal batteries. However, the charge compatibility within EDL is destroyed by the spatiotemporal discord between...
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DOI: 10.1039/D5EE01092F, PaperSinan Zheng, Yang Wang, Bin Luo, Kun Zhang, Leilei Sun, Zhean Bao, Guosheng Duan, Dinghao Chen, Hanwei Hu, Jingyun Huang, Zhizhen Ye
The dynamic reconstruction of electric double layers (EDLs) holds the key to stabilizing aqueous Zn metal batteries. However, the charge compatibility within EDL is destroyed by the spatiotemporal discord between...
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Wearing “Body Armor” on Zinc anodes for Robust Aqueous Zinc-ion Batteries
Energy Environ. Sci., 2025, Accepted Manuscript
DOI: 10.1039/D4EE05757K, PaperQunhao Wang, Xueyong Deng, Xiaolin Xue, Jian Zhang, Jiangqi Zhao, Zengyan Sui, Yuefei Zou, Longbo Luo, Wei Zhang, Xiangyang Liu, Canhui Lu
Rechargeable aqueous zinc batteries (ZIBs) are a promising device for sustainable energy storage, yet their application is hindered by uncontrollable Zn dendrite growth and parasitic reactions. Herein, a flexible membrane...
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DOI: 10.1039/D4EE05757K, PaperQunhao Wang, Xueyong Deng, Xiaolin Xue, Jian Zhang, Jiangqi Zhao, Zengyan Sui, Yuefei Zou, Longbo Luo, Wei Zhang, Xiangyang Liu, Canhui Lu
Rechargeable aqueous zinc batteries (ZIBs) are a promising device for sustainable energy storage, yet their application is hindered by uncontrollable Zn dendrite growth and parasitic reactions. Herein, a flexible membrane...
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Single Ion Conductive “Plasticine-Like” Solid Electrolyte Combined with Modulated D-Band Center of Interfacial Zinc Atoms for Highly Reversible Zinc Metal Anode
Energy Environ. Sci., 2025, Accepted Manuscript
DOI: 10.1039/D5EE00737B, PaperKang Yan, Yongbo Fan, Xueya Yang, Xinyu Wang, Shengmei Chen, Weijia Wang, Mingchang Zhang, Huiqing Fan, Longtao Ma
Highly concentrated salts, like 30 m ZnCl₂, can reduce free water molecules in aqueous electrolytes but also increase acidity, causing severe acid-catalyzed corrosion of the Zn anode, current collector, and...
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DOI: 10.1039/D5EE00737B, PaperKang Yan, Yongbo Fan, Xueya Yang, Xinyu Wang, Shengmei Chen, Weijia Wang, Mingchang Zhang, Huiqing Fan, Longtao Ma
Highly concentrated salts, like 30 m ZnCl₂, can reduce free water molecules in aqueous electrolytes but also increase acidity, causing severe acid-catalyzed corrosion of the Zn anode, current collector, and...
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Achieving 20% Efficiency for Binary Organic Solar Cells with Suppressed Non-radiative Recombination via Triphenylamine Halides†
Energy Environ. Sci., 2025, Accepted Manuscript
DOI: 10.1039/D5EE01165E, PaperJunjie Zhang, Xiaopeng Duan, Xiaoming Li, Guangkuo Dai, Jiawei Deng, Xunchang Wang, Jiawei Qiao, Hanzhi Wu, Liming Liu, Haodong Huang, Sha Liu, Jun Yan, Huotian Zhang, Xiao-Tao Hao, Renqiang Yang, Feng Gao, Yanming Sun
Minimizing energy loss has been identified as an effective approach to achieve further efficiency breakthroughs in organic solar cells (OSCs), and the main loss channel can be attributed to non-radiative...
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DOI: 10.1039/D5EE01165E, PaperJunjie Zhang, Xiaopeng Duan, Xiaoming Li, Guangkuo Dai, Jiawei Deng, Xunchang Wang, Jiawei Qiao, Hanzhi Wu, Liming Liu, Haodong Huang, Sha Liu, Jun Yan, Huotian Zhang, Xiao-Tao Hao, Renqiang Yang, Feng Gao, Yanming Sun
Minimizing energy loss has been identified as an effective approach to achieve further efficiency breakthroughs in organic solar cells (OSCs), and the main loss channel can be attributed to non-radiative...
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Amorphous Indium-Zinc Oxide Layer with Transport and Protective Dual-Function for High-Efficiency Semitransparent and Tandem Sb2(S,Se)3 Solar Cells
Energy Environ. Sci., 2025, Accepted Manuscript
DOI: 10.1039/D4EE04699D, PaperJunjie Yang, Jianyu Li, Yuehao Gu, Rongfeng Tang, Lei Huang, Zhiyuan Cai, Bo Che, Qi Zhao, Shuwei Sheng, Hong Wang, Changfei Zhu, Tao Chen
Environmentally friendly Sb2(S,Se)3 with excellent optoelectronic properties is considered to be a promising light-harvesting material, which can be applied to highly efficient semitransparent solar cells when well coupled with a...
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DOI: 10.1039/D4EE04699D, PaperJunjie Yang, Jianyu Li, Yuehao Gu, Rongfeng Tang, Lei Huang, Zhiyuan Cai, Bo Che, Qi Zhao, Shuwei Sheng, Hong Wang, Changfei Zhu, Tao Chen
Environmentally friendly Sb2(S,Se)3 with excellent optoelectronic properties is considered to be a promising light-harvesting material, which can be applied to highly efficient semitransparent solar cells when well coupled with a...
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Dielectric Constant Engineering of Nonfullerene Acceptors Enables a Record Fill Factor of 83.58% and a High Efficiency of 20.80% in Organic Solar Cells
Energy Environ. Sci., 2025, Accepted Manuscript
DOI: 10.1039/D5EE00101C, PaperJunwei Dong, Yinfeng Li, Chentong Liao, Xiaopeng Xu, Liyang Yu, Ruipeng Li, Qiang Peng
Organic solar cells (OSCs) have shown promise with power conversion efficiencies (PCEs) exceeding 20%, but their performance still lags behind silicon-based and hybrid perovskite solar cells. A critical limitation is...
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DOI: 10.1039/D5EE00101C, PaperJunwei Dong, Yinfeng Li, Chentong Liao, Xiaopeng Xu, Liyang Yu, Ruipeng Li, Qiang Peng
Organic solar cells (OSCs) have shown promise with power conversion efficiencies (PCEs) exceeding 20%, but their performance still lags behind silicon-based and hybrid perovskite solar cells. A critical limitation is...
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Importance of hydrogen oxidation reaction current in quantifying hydrogen crossover in PEM water electrolyzers at high differential pressure
Energy Environ. Sci., 2025, Advance Article
DOI: 10.1039/D5EE00048C, Communication Open Access   This article is licensed under a Creative Commons Attribution-NonCommercial 3.0 Unported Licence.Ramchandra Gawas, Douglas I. Kushner, Xiong Peng, Rangachary Mukundan
This work employs online gas chromatography and hydrogen oxidation current measurements for accurate quantification of the hydrogen crossover rates in proton exchange membrane water electrolyzers operating at high differential pressure.
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DOI: 10.1039/D5EE00048C, Communication Open Access   This article is licensed under a Creative Commons Attribution-NonCommercial 3.0 Unported Licence.Ramchandra Gawas, Douglas I. Kushner, Xiong Peng, Rangachary Mukundan
This work employs online gas chromatography and hydrogen oxidation current measurements for accurate quantification of the hydrogen crossover rates in proton exchange membrane water electrolyzers operating at high differential pressure.
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Ballistic ion transport through hierarchically-ordered-structure polymer binder
Energy Environ. Sci., 2025, Advance Article
DOI: 10.1039/D4EE06071G, PaperDefu Li, Chen Fang, Santosh Thapa, Hadas Sternlicht, Gi-Hyeok Lee, Faiz Ahmed, Xiuyu Jin, Qiusu Miao, Raynald Giovine, Wanli Yang, Andrew Minor, Yang-Tse Cheng, Gao Liu
Achieving ballistic ion transport in a mixed electronic-ionic conductive polymer, its hierarchically ordered structure (HOS) facilitates ion diffusion and results in solid-state Li+ conductivity in the range of 10−4 to 10−3 S cm−1 from −20 to 70 °C.
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DOI: 10.1039/D4EE06071G, PaperDefu Li, Chen Fang, Santosh Thapa, Hadas Sternlicht, Gi-Hyeok Lee, Faiz Ahmed, Xiuyu Jin, Qiusu Miao, Raynald Giovine, Wanli Yang, Andrew Minor, Yang-Tse Cheng, Gao Liu
Achieving ballistic ion transport in a mixed electronic-ionic conductive polymer, its hierarchically ordered structure (HOS) facilitates ion diffusion and results in solid-state Li+ conductivity in the range of 10−4 to 10−3 S cm−1 from −20 to 70 °C.
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Reviving ether-based electrolytes for sodium-ion batteries
Energy Environ. Sci., 2025, Accepted Manuscript
DOI: 10.1039/D5EE00725A, Review Article Open Access   This article is licensed under a Creative Commons Attribution-NonCommercial 3.0 Unported Licence.Fangyuan Cheng, Jun Hu, Wen Zhang, Peng Yu, Xueliang Sun, Jian Peng, Baiyu Guo
The development of ether-based electrolytes has significant challenges, primarily caused by the irreversible co-intercalation of ether and Li+ into commercial graphite, which excluded ether from use in commercial lithium-ion batteries...
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DOI: 10.1039/D5EE00725A, Review Article Open Access   This article is licensed under a Creative Commons Attribution-NonCommercial 3.0 Unported Licence.Fangyuan Cheng, Jun Hu, Wen Zhang, Peng Yu, Xueliang Sun, Jian Peng, Baiyu Guo
The development of ether-based electrolytes has significant challenges, primarily caused by the irreversible co-intercalation of ether and Li+ into commercial graphite, which excluded ether from use in commercial lithium-ion batteries...
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